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Overscan refers to do a degree of cropping on all four sides of the image done by old tube tvs. It does not apply to HD. What you're seeing on the other hand is proper anamorphic widescreen (except maybe with those 1.66:1 titles, they should have small black bars on the left and right sides...

In the case of Thunderball, the windowboxing was also present on the 1999 dvd so its possible it might actually be that way on the original print.