Not a big fan of (North American) TV cartoons from the 1980s, but I'd buy it if they included some episodes of Beetlejuice (provided they're not the exact same cartoons already released on the Beetlejuice movie SE), The Charlie Brown and Snoopy Show (since Warner owns the video rights to the Peanuts specials, maybe they could release this), Pac-Man, Yogi's Treasure Hunt and the 13 Ghosts of Scooby-Doo (the latter two are of interest to me because they feature the work of future big names like Tiny Toons/Animaniacs/Pinky & The Brain/Freakazoid!/Batman: The Animated Series producer Tom Ruegger and Angry Beavers creator Mitch Schauer).
If they could come to terms with the respective video game companies (if need be), they might as well include at least a few cartoons from Saturday Supercade, if only because characters like Mario and Donkey Kong are uber-well-known.
It also might be interesting if they include a few cartoons from the 1988 New Yogi Bear Show.
Filmation's the Tom & Jerry Comedy Hour is like the "Plan 9 from Outer Space" of animation: so bad it's actually kinda funny. And hopefully, if included, someone (like the MST3K veterans who do Rifftrax) could make an audio commentary MST3K-style on an MP3.
Anybody remember Turbo Teen? It only sits out in my mind because Cartoon Network used to do ads that mocked it, which should tell you all you need to know about its quality. But, I suppose it should be included simply because it's almost achieved a certain level of infamy.
And call me crazy, but if they included an episode of the Snorks, I wouldn't oppose.
But what would really excite would be a 90s Saturday Morning Cartoons set. I'm very partial to the WB and Cartoon Network shows of the '90s, like Tiny Toons, Animaniacs, Taz-Mania, 2 Stupid Dogs, What-A-Cartoon!, Dexter's Lab, Cow & Chicken, etc.